Abstract
Two diazaporphyrin (DAP)-porphyrin hetero dimers, in
β-meso and β-β configurations, were prepared to
study their photoinduced intramolecular electron transfer
properties. The two meso nitrogen atoms in the porphyrin ring of DAP
change its redox potential making DAP more easily reduced, compared to
its porphyrin counterpart. A charge-transfer from porphyrin to DAP in
both hetero dimers was verified by versatile optical spectroscopic
methods. The steady-state fluorescence spectra indicated an efficient
intramolecular exciplex formation for both dimers. For the
β-meso dimer, ultrafast time resolved spectroscopic
methods revealed the sub-picosecond formation of two types of primary
short-living (1–18 ps) intramolecular exciplexes, which relaxed in
toluene to form a long-living final exciplex (1.4 ns) followed by a
longer-living charge transfer complex (> 5ns). However, in
benzonitrile the lifetime of the final exciplex was longer (660 ps) as
was that of the charge transfer complex (180 ps). The β-β
analogue formed similar short-living exciplexes in both solvents, but
the final exciplex and the charge transfer state had significantly
shorter lifetimes. The electrochemical redox potential measurements
and DFT calculations supported the proposed mechanism.