Abstract
Solvent models and sampling schemes for obtaining average physical
properties for molecules in solution utilizing combined quantum
mechanical / molecular mechanical (QM/MM) method are reviewed and a
new sampling scheme of ours is presented. In the new scheme, we sample
the structure of the solute molecule and solvent molecules
separately. First, we execute a QM/MM MD simulation, where we sample
the solute molecule in solution. Next, we choose random solute
structures from this simulation and perform classical MD simulation
for each chosen solute structure with its geometry fixed. This new
scheme allows us to sample the solute molecule quantum mechanically
and sample many solvent structures. This scheme is combined with the
generalized-multiconfigurational perturbation theory and applied to
study the absorption spectra of Coumarin 120 in water. We succeeded in
constructing the absorption spectra and in realizing the red shift of
the absorption spectra found in polar solvents. We found that the
umbrella-like open-close motion of the amino group of the coumarin
plays an important role in the broadening of the spectra, whereas the
red shift of the peak was caused by the solvation structure of the
amino group.